Two-dimensional confinement of 3d{1} electrons in LaTiO_{3}/LaAlO{3} multilayers.

نویسندگان

  • S S A Seo
  • M J Han
  • G W J Hassink
  • W S Choi
  • S J Moon
  • J S Kim
  • T Susaki
  • Y S Lee
  • J Yu
  • C Bernhard
  • H Y Hwang
  • G Rijnders
  • D H A Blank
  • B Keimer
  • T W Noh
چکیده

We report spectroscopic ellipsometry measurements of the anisotropy of the interband transitions parallel and perpendicular to the planes of (LaTiO3)n(LaAlO3)5 multilayers with n=1-3. These provide direct information about the electronic structure of the two-dimensional (2D) 3d{1} state of the Ti ions. In combination with local density approximation, including a Hubbard U calculation, we suggest that 2D confinement in the TiO2 slabs lifts the degeneracy of the t{2g} states leaving only the planar d{xy} orbitals occupied. We outline that these multilayers can serve as a model system for the study of the t{2g} 2D Hubbard model.

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عنوان ژورنال:
  • Physical review letters

دوره 104 3  شماره 

صفحات  -

تاریخ انتشار 2010